Instructions
Play through "Castlevania: Harmony of Despair" with a friend. Kill monsters, loot items and progress through the game's early levels until you encounter the first boss, Gergoth.
Fight Gergoth until he is extremely weak. Once he has reached around 10% of his normal health, you and your friend should begin executing Dual Crush attacks.
Stand next to your friend and press the right-trigger button to initiate a Dual Crush.
Ask your friend to hit the right trigger just as you initiate the attack. Your friend must confirm the attack to execute a Dual Crush.
Repeat this process until the boss has been slain by a Dual Crush and you will earn the "Grim Synergy" achievement.